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Collection (1821-2000, undated [bulk: 1989-2000]) of correspondence, family histories, genealogical charts, copies of deeds, cemetery records, Bible records, miscellany and oversized materials relating to Christopher DeGraffenried, also known as Baron Christoph von Graffenried, who established a colony of Swiss and Palatine emigrants at New Bern, North Carolina, in 1710; and also relating to his ancestors and descendants and the DeGraffenried Association, of Gulfport, Mississippi and San Antonio, Texas, which was established to preserve the family history and to maintain contact between family members; in English, German, Italian, and French language.

Papers (1916-1926) including correspondence, flight training material, orders, letters, etc.

Papers of Merrill Moore (1929–1987, undated) documenting the life and literary career of the noted Columbia, Tennessee-born American poet, physician and psychiatrist, who became a leader and spokesman for the Fugitive Group of Southern poets that included Robert Penn Warren and Allen Tate, among others; including correspondence, manuscript materials, printed materials and loose manuscript materials from the Stuart Wright Book Collection.

Papers (April 1942 – April 1943, undated) consisting mainly of photographic prints originally belonging to a photograph album compiled by David Y. Taylor, documenting progress on several troubled U.S. Navy construction project contracts to build shipyards and ship repair facilities in the vicinity of Charleston, South Carolina, and Savannah, Georgia; including contracts awarded to Charleston Shipbuilding and Dry Dock Company, the Clifford F. MacEvoy Company, the Savannah Machine & Foundry Company, and to its Shipbuilding Division; including projects to construct plant facilities, dry docks and floating dry docks, caissons, retaining walls, coffer dams, graving docks, piers, wharfs, pilings, and bulkheads, etc.; the photographs also show work crews, including racially integrated crews, and equipment, including: railroads, docks, buildings, trucks, cranes, and pile drivers; also including the leather-bound front cover of the original photograph album.

Papers (1907-(1930)-1965) including correspondence, minutes, reports, clippings, photographs, broadsides, pamphlets, press releases, radio scripts, post cards, genealogy, and miscellany.

Papers (1863-1864) consisting of diaries with activities of battle.

Papers (1930-1949) including correspondence; agriculture and gardening; export of flowers and vegetables; travel account; letters and miscellaneous.

Papers (1927-1969, undated) including correspondence, memoirs, reports, flight records, flight log, speeches, etc. relating to the career of pioneer aviator and US Army Air Corps general during and after World War II.

Records (2008-2016) document the history of the Perry-Weston Educational and Cultural Institute, Inc., from its founding in 2008 by Mr. C. Rudolph Knight, Dr. Florence A. Armstrong, and Dr. Lawrence W. S. Auld to promote African American history, genealogy, culture, and arts, particularly in Edgecombe County (Princeville and Tarboro) and North Carolina, until its dissolution in 2016. Included are programs, invitations, circulars, posters, correspondence, clippings, and articles of incorporation and dissolution that document exhibits, historic talks and presentations, tours, a Nonagenarian Tea, and publications.

Papers (1941-1970) of member of U. S. Naval Academy Class of 1941, including correspondence, orders, citations, an informal log of his naval service, 1941-1947, a photographs, and miscellany relating to his service aboard the destroyers USS LEA and the USS WADSWORTH during World War II and his postwar naval career.

A collection that contains 57 diaries kept by Edward Dunham Robie (1831-1911) who was a naval engineer, inventor and a U.S. naval officer during the American Civil War.

Papers of ECU professor Dr. Richard C. Todd containing awards for his service at ECU, information about the establishment of the Richard and Clauda Todd endowment, postcards, and materials from his alma mater Millersville State Teachers College, and materials in relation to his publication Confederate Finance.

Collection (1963-1988, n.d. [Bulk: 1980-1988]) of photographic prints and negatives of city government officials and employees, buildings and activities taken in and around Greenville, North Carolina, for the City of Greenville (NC) Public Works Office.

Papers (1758-1953, undated) including correspondence, financial records, land records, remedy for eye problem, laundry, haircuts, Christian club, etc. 372 items.

Papers (1791, 1846-1941) including correspondence, diaries, visitation books, account books, memoranda books, financial papers, minute books, photographs, land records and miscellaneous.