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James Lafayette Whitehurst was born on November 5, 1861 in Bethel Township, Pitt County, North Carolina. His family stayed in Pitt County or moved to Martin County, North Carolina. The collection contains a book written by Margaret Ann Whitehurst in 2006 containing blank spaces to fill in births, deaths, and marriages. There are also photos of the Whitehurst family generations 1-6.

Papers (1920-1953) including correspondence, membership lists, financial records, meetings, essay, newspapers, magazines, clippings, scrapbook, reports, Lee Jackson Day celebration, etc.

Papers (1869, 1908, 1736, 1933-1956) consisting of correspondence, legal records, genealogical records, pamphlets, clippings, photographs and miscellaneous.

Administrative records of The William E. Laupus Health Sciences Library includes papers, publications, and photographs.

Papers (1941-1945) related to Shipfitter First Class Mariano Albert Bellitteri's service on board the USS Miami including radio press releases, newsletter, yearbook, photographs, discharge papers, "plank ownership" certificate, and a brass ashtray from the USS Miami.

The Louis Orr Collection contains a set of forty-eight prints of the original fifty-one print set (and one replacement print) made from etchings of North Carolina historical landmarks and architectural sites. The etchings were created from 1939 to 1952 by artist Louis Orr, a world-renown etcher, at the behest of North Carolina resident Robert Lee Humber who wanted to preserve North Carolina's heritage by providing the artwork to schools, colleges, public libraries and institutions throughout the state.

Letters (August 1917-August 13, 1919) written by Mary and Gordon Robertson of Africa Inland Mission while they were working in the Belgian Congo. They described their work providing education and religious training, how World War I was affecting the area, indigenous customs, and the practice of cannibalism which was still in existence in some villages.

Papers (1960-1962, 1986, undated) compiled by Doris M. Cromartie, during her service as vice chair of the executive committee of the Democratic Women of North Carolina, including correspondence, lists of workers, by-laws, newsletter, articles, and miscellaneous materials pertaining to Democratic Party activities in North Carolina.

Papers (1864-1958 undated) of Rocky Mount, North Carolina, lawyer, judge, legislator, and gubernatorial candidate Richard Tillman Fountain consisting of correspondence, report, clippings, newspapers, law practice documents, letters, pamphlets, photographs, clippings, scrapbooks, and reports.

Papers (1762-1902, undated) documenting the life of the Noble family from the Chicod Township of Pitt County and the Creeping Swamp and Swift Creek areas of Craven County. The bulk of the collection includes material related to the activities of Celina Clark Noble (1829-) and her family and includes land records, land description and surveys, promissory notes, mortgages and other legal papers, bank notes, ballads, financial papers, receipts, etc. Also included is the Civil War correspondence (1864-1865) of Corporal E. E. (Evans Everette) Noble (1829-1895) of the 67th Regiment North Carolina Infantry to his wife Susan J. Noble (1837-1873) while serving throughout Eastern North Carolina.

Collection contains a newspaper clipping (6/10/1923) entitled "Christian Church Growth in 20 Years Proud Record, Dedication Services Sunday" from the Greenville, North Carolina, Daily Reflector.

Collection (ca. 1987 – 2004) of maps, photographs, correspondence, genealogical research on the descendents of Shadrack Allen, Sr., newspaper clippings, photocopies, and other printed sources, including transcriptions of manuscript materials, concerning President George Washington's historic "Southern Tour" of 1791, focusing especially on those events occurring in Pitt County, North Carolina.

Papers (2/23/1862 - 12/26/1868) consisting of a pocket notebook belonging to James H. Mills, Sergeant of Company I, 44th Regiment North Carolina Troops, the "Eastern Tigers," a unit recruited in Pitt County, including orders, inventories, muster and supplies lists related to the Civil War and a few post-war account records.

Papers (1944-1987) including correspondence, an article, biographical data, personnel list, comments, sketch, etc.